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AbstractThis article reports the systematic functionalization of FIrpic (1) with solubilizing alkyl groups (complexes 2 4) or mesityl groups (complexes 5 and 6). Complex 5 is shown to offer significant advantages over FIrpic (1) in terms of performance of sky blue polymer based phosphorescent organic light emitting diodes (PhOLEDs) with a solution processed emitting layer (maxEL 477 nm for 5). Devices with 5 doped into poly(vinylcarbazole) (PVK):OXD 7 gave a maximum luminous efficiency of 19.1 cd A 1 at a brightness of 5455 cd m2 with EQE 8.7%.

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